Excellent coordination requires really only one thing: when the thumb makes its rotational crossing, notice what type of rotation is required in the other hand at the same time. Practice that. Simple.
Well, at first it's a little like trying to pat your head and rub your tummy at the same time. Exaggerate the movements, first in one hand then the other. Then put the hands together. Slowly. Deliberately. Breathe. Don't panic. Keep in mind that this is an underlying tool and becomes so tiny in speed as to be invisible.
Notice that in the video I add an in/out shaping to the scale. Ignore this at first until the coordination is well worked-in. Remember, my demonstration is greatly exaggerated.
Now exhale.